The difficulty of tasking myself to pinpoint some songs as my favorites nearly taxed all of my strength away. :p So without further ado, here are my favorites:
"Orinoco Flow" sends me across the sea to a land of a pure magic and enchantment. Every time I listen to it I feel as though I'm stepping through Narnia's wardrobe into a new land.
"The Call" is without a doubt one of my all time favorites. Chloe in the beginning *shudders*, it is just an indescribable feeling, we'll leave it at that. Lynn just rolls her flowing voice into the mix and seals the deal. "The Call" is one of my favorite songs lyrics wise too. Plus, I also have the amazing DVD version in the back of my head that always brings a "wow" factor.
"Nil Se'n La" is a guaranteed smile no matter how I feel. The version with Lisa Lambe is my personal favorite (though Lynn and Alex are just as beautiful) mainly because of Lisa line, "I can see the starlight shining." It gives me a Cheshire Cat smile
Listen for yourself at about the 1:26 mark
http://www.youtube.com/watch?v=KBymZCmW6KA "Dulaman" is another wonderful one. I discovered Meav's version first so I'm a bit partial to that one. Meav's combo of eyes, motions, and voice are a killer deal. Lisa Lambe spins the song into a more "fun" or even "bouncy" version, which is just as fantastical.
I could go on and on until I've listed every song they've ever sung....but I give you my ALL TIME favorite songs....:p